Bioshock is known for using real world music in some fantastic ways and Infinite is no different. For me personally it was the moment when Elizabeth first opens a Tear in front of you and you see a modern day city. The Tears For Fears song Everybody Wants To Rule The World plays before the Tear shuts. It was a great revelatory moment of, "Holy shit, she's opening holes in both space and time."
If that wasn't cool enough later in the game there's a phonograph that plays an old-timey rendition of the same song. I'm honestly not sure if it was indeed the original version of it. I remember thinking that the damage to the timeline must be so severe that the song was made before Tears For Fears even existed. It's more possible that I'm just not very well acquainted with that era of music.
I've heard a number of recognizable songs and scores so I wanted to hear from the community. What was the best use of a licensed song in your opinion?