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Unlike Ornstein, Smough was not allowed to join the ranks of Gwyn's Knights because of his custom of pulverizing his victims' bones and adding them to his meals.
The player fights him alongside Ornstein. Smough uses attacks which utilize his powerful hammer and his enormous weight by occasionally doing a butt stomp - an ability which Ornstein will use if Smough is killed first.
If he is defeated last in battle, his armor will be available for purchase from Domnhall of Zena and his hammer can be crafted from his soul. Smough's armor set is one of the strongest in the game.
This set cannot be improved.