DS9 is great for its characters and its political drama. It has very few unwatchable episodes, but some of it feels a bit redundant because it focuses on the Bajor/Cardassia angle so much.
TNG is of course a classic, with a lot of great episodes but also quite a few hammy and unwatchable ones. I feel like people generally put on their rosiest of colored glasses when talking about TNG.
Voyager is a little inferior to either DS9 or TNG just by the virtue of its characters and writing, but it's still very good. It has its share of very memorable episodes and characters. If you haven't seen Voyager, you should rectify that.
Enterprise is sort of a curiosity. It's so different from all the others. I'd watch a few episodes and see if it hooks you. I stopped watching halfway through and haven't gone back.
TOS is a historical curiosity, worth watching every now and again. A few classic episodes hold up today.
My personal favorite is DS9, but I can see arguments for TNG or even Voyager.
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