Persona 4 seems to be all the rage on the PS2 these days. Never played it, but you could check it out.
God of War 1 and 2 don't get old very easily. You've probably already played them, but they don't get old.
Ratchet and Clank 2 and 3 don't get old either. Also the Jak and Daxter games.
Silent Hill 2, I hear, is quite a good game.
The original Half-Life is on PS2.
The original Deus Ex was ported to PS2, though I don't know if it was gimped or not.
I liked Goldeneye Rogue Agent way back when.
Ico/Shadow of the Colossus if you haven't yet.
Mega Man X Collection, if you want something classic and awesome.
The other two POP games, of course.
Devil May Cry 3 is nuckin' futs.
Dragonball Z Budokai 3 is a fun little fighter.
Kingdom Hearts 1 and 2.
Gran Turismo 4
Grand Theft Auto III/Vice City/San Andreas/Liberty City Stories
...well, there's a good variety of pretty much everything. You ought to be able to find something in there to your tastes.
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