Persona 4 Golden is definitely the best game on the system. It doesn't satisfy your request for crafting (there basically isn't any - you sell the materials you loot to a NPC and then items get added to his vendor list for you to buy), but it has a lot of loot, very deep combat, excellent characters and story.
Alternately, there is Disgaea 4: A Promise Revisited. It's a tactical RPG, in that you're moving characters around on a battle grid, and it has some very unique features. For example, the item dungeon system. You can "enter" a weapon (which basically places you into a dungeon) and the weapon will be improved based on how far you get in said dungeon. Tons of characters and items. Amusing story. No crafting, I think, though.
For crafting in a RPG, you'll have to look at the Monster Hunter clones - Soul Sacrifice Delta is really good. I never beat it, so I'm a little fuzzy on the story, but you play as a sorcerer and the loot comes in the form of spells you can equip, in addition to equipping an ultimate spell (that has a variety of interesting effects on use) and, if I remember correctly, special glyphs/gear for your character's arm.
Another Monster Hunter clone that's alright is Freedom Wars. It has a really interesting story, set in the year 102014 - you start by losing your memory, which is a crime apparently, and are sentenced to 1,000,000 of prison. You then have to fight monsters to decrease that sentence. Additionally, basically everything you do is a crime until you unlock the privilege of being able to do said action - such as lying down. Or walking near a member of the opposite gender. I haven't gotten very far, so someone else will have to enlighten you as to what the crafting is like. Combat seems fun - you get a whip-thing that lets you jump onto the large enemies and hack at places other then their ankles. The whip-thing can apparently also be used to drag the monsters to the ground. Unlike most Monster Hunter games, you aren't restricted to only one weapon (usually melee) - you can also equip more modern weapons, such as assault rifles.
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