I would love, love, love it if he wrote a comedic collection of anecdotes called Tales from the Compound about his quasi-shady exploits living with a bunch of other people last decade, what with the violent parties and turned over cars and police raids. When he has spoken about that part of his life he's always relayed it in an engaging and intriguing manner. He knows how to structure and deliver information in a way that's just naturally funny.
Wouldn't 'gamer comedy' be huge if it were a thing?
And true, anecdotes are funny but wear out quick. I think good comedy is about observation and reacting. If you see things in a funny way, you can be a comedian and theoretically always have access to material. And Jeff makes things just seem funny.