With Street Fighter II Turbo HD Remix's awesome music. Just put my coontroller down to air guitar solo that insane section. Pity I'm awful at the game.
 I do wish this song was on Rock Band.
 
How about you guys? Anything on a game that made you want to put your controller down and just replay it over and over again because of its sheer awesomeness?

Yes! In Street Fighter Alpha III, one of the stage's music is just beyond awesome. I forgot which one unfortunately, I think it was the NYC one with the Jazzy music.
 
EDIT: It's Street Fight III: Final Strike.

The music in Sonic 3(I think) that is in the Battery Zone level.  Some of the best game music I have ever heard.

I really don't understand the "I love this song so I wish it was in Rockband"  phenomenon.

What that game was missing was the intro from Street Fighter 2 where the black guy gets punched out by the white guy.  Fucking great intro with great music.

I've got the SFIITHDR soundtrack on my computer and I didn't even play the demo. Someone just linked me to a video on YouTube and the music was so, so good. Far better than Street Fighter IV's soundtrack which ranged from boring and unnoticeable to annoying as shit.

Chrono Trigger has a great soundtrack.

I play the game with the original music, which is better imo. 

 @eroticfishcake: 
 
It is true, he just chose not to put his name on it due to the final product being far from his expectations. (lame MD/Genesis audio chip) 
 
http://www.giantbomb.com/sonic-the-hedgehog-3/61-4628/micheal-jackson-worked-on-sonic-3/35-274873/#4

With all of this talk concerning Street Fighter and soundtracks, I now have the Indestructible song from Street Fighter IV stuck in my head. Thanks guys!
 
As far as soundtracks that I enjoy listening to, I'd have to go with Katamari Damacy. I finished the game in no time flat and never really had any desire to play it again - except for those rare occasions when someone was over who had not yet experienced it - but I still enjoy listening to the soundtrack every once in a while. Good stuff. The Ouendan soundtrack had some great songs as well. Of course, it would be an error if I didn't mention Mega Man 2 and Contra. Can't believe I almost forgot those.

I remember liking the F-Zero X soundtrack.

I thought you meant you fell in love with a person.lol

I love the remix of Zangief's theme in SSF2THD.

The track that plays in Mega Man Battle Network 4's Undernet. I would to go there, put down the game, and just listen to the music. Man, the Battle Network series had some crazy good tunes.
  

Battletoads pause music > all other music.

"Indestructible!
I wont let nobody take me down!
Indestructible!
Nothing's gonna stop me now!".
 
No, seriously. Seriously. I fucking love that song. It's so horrible that it's amazing.

Secret of mana had some great music i think. 
  

   
I also liked some of the music from metal gear and i still think this song on this other youtube video was either in metal gear or one that sounded very like it.

Love the music in Super Mario Galaxy.  It's just pure awesome.  Like they say "You can't beat 100%" and that's what this soundtrack is.
 

" Chrono Trigger has a great soundtrack. "

Wipeout HD FURY has an awesome soundtrack. I can help but nod along to the music even when I'm carving my ship into the wall.

" The music in Sonic 3(I think) that is in the Battery Zone level.  Some of the best game music I have ever heard. "

Thought I might upload a few more bits of music which I really enjoy from games.
 
 

I just remembered my favorite soundtrack: FF VII.  Brings back memories...