I buy multi-platform games games on 360 primarily because they often run/look better but also for playing with friends via Live. Exclusives I've enjoyed but far from complete list:
Alan Wake
Gears of War Series
Saints Row
Halo Series
Lost Odyssey
Banjo Kazooie: Nuts & Bolts
Dance Central Series
The Gunstringer
Fable 2
Forza Series
Chrome Hounds
Dead or Alive 4
Culdcept Saga
Earth Defense Force 2017
Crackdown
Deathsmiles II
Operation Darkness
Raiden IV
-------- XBLA ---------
Shadow Complex
Assault Heroes Series
Bomberman Live
Explosion Man Series
Bangaioh HD: Missile Fury
Guardian Heroes
Soulcalibur
Radiant Silvergun
Omega 5
Virtual On: Oratorio Tangram
R-Type: Dimensions
-------- If PC doesn't count --------
Mass Effect Series
Condemned: Criminal Origins
Insanely Twisted Shadow Planet
Bastion
Monday Night Combat
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