I can't really think of any ways that Fallout 3 is better than New Vegas.
Even in terms of gameplay and RPG mechanics New Vegas is much superior to the rather broken, poorly balanced mess that was Fallout 3. New Vegas actually has some variety to character builds and different armour categories are actually viable. In Fallout 3 all characters can easily become 10 in all stats, 100 in all skills demi-gods in power armour as no other armour types are really viable.
New Vegas cut out some of the unwarrented or somewhat broken perks and made it so you get them every 2 levels, which prevents the player from being so flooded with perks that there is only one way to correctly build/play a character as was the case in fallout 3.
In terms of narrative and setting there really is no contest, New Vegas presents a rich, extensive setting based on years of work from the cancelled Van Buren project. Every faction has both good and bad points. Fallout 3 felt more like a fallout fan-fiction; morally pure and good brotherhood paladins vs. evil Enclave. It really wasn't very true to the more grey tone of the setting.
As for a comparison of the choices and number of potential endings, there are all of about 7 choices (right at the end of the game) that Fallout 3 factors in towards your ending. Fallout New Vegas (without addons) has 176 choices/variables for the ending, which are ticked off throughout the course of the game. Technically around 288 if you include all the addons assorted endings. So New Vegas provides a lot more information and closure.
Fallout New Vegas is a much deeper and well written experience. The only issue it really faced was bugs on launch but that has been largely resolved now. I enjoyed Fallout 3 at the time, but after playing New Vegas so much I really can't go back.
Anyway as for mods that don't really drastically alter the experience beyond a visual tweak perhaps better textures might be a good idea?
Also i'd probably recommend playing the various DLC in order as there is actually an overarching plot thread that is hinted at through all of them and is the focus of the final DLC addon.
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