Sky UI for sure
Realistic Colors Realistic Nights or Climates of Tamriel to improve visuals
Xenius Character Enhancement to improve the look of your character and NPC's
Dynamic Merchants is pretty good, makes selling stuff a bit less of a pain in the arse
Reduced NPC Greeting if you get pissed off with NPC's constantly talking to you.
Static Mesh Improvement Mod makes a big difference to the visuals. It takes stuff that would normally be flat bitmaps(?) and makes them into 3D meshes.
Dynavison and The Imaginator are good. Dynavison adds dynamic depth of field and you can use Imaginator to change colours, contrast, brightness etc in real time.
Categorized Favourites Menu. Get this one! Makes a massive improvement to the favourites menu, especially paired with Better Sorting.
Warzones is fun. It adds lots of random battles between various factions all over the map. Some of the battles are huge.
So many great mods. Go to Skyrim Nexus, go to files and check out the top files. Some of the mods there are pretty much essential.
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