I'm pretty sure it was part of the second Big Live Live Show Live. Not sure about when in the video it is but there you go.
Edit- Found it (12:05)
Edit 2- Never mind that wasn't it but I'm pretty sure it was caught on tape somewhere during the BLLSL 2 so maybe watch the whole thing and see if you find it.
Edit 3- Also Will Smiths hilarious "O" face at 29:34
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