OG Dragonball or Yu Yu Hakusho are my votes, for sure. The only problem with Yu Yu is that it kinda drops off in quality after the Dark Tournament arc, I think. It's still pretty good, but it definitely never reaches the highs of that arc again.
Outside that, I think shorter stuff like FLCL could be fun, or Gurren Lagann I think could be the right level of light-hearted ridiculousness that Jeff and Dan might enjoy.
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