I "only" have a PCIe3 SSD, but my opinion would be no.
Here's my reasoning, which I used last year when upgrading:
The upgrade from HDD to SSD is huge. It is a 10x speed increase in load times, which returns into insanely faster boot speeds (Windows10 is fickle, but if you reboot often 10 seconds is about the region you end up with), really snappy desktop performance, where every app opens in a few seconds. And load times in games that are often between 0.1x and 0.5x of what they were before SSDs.
The upgrade from SATA to NVME is incremental. It is roughly a doubling, and maybe shaves a second here and there in realtime performance.
To spend additional money even faster NVME seems like it is better spent elsewhere in the system. Or doubling the SSD size instead, which means that you spend less time managing drive space.
Adding additional faster load times only helps if that is still the bottleneck. And even if it is, if a single player games goes from a 30 second load to a 5 second load that's great. The difference between a 5s load and a 3s load is much less impactful.
Of course in most multiplayer games load times matter even less because you're then stuck waiting for other people to load in.
The new console generation is able to take advantage of very high throughput SSDs because every console has it. This makes for really different restrictions about what can be expected to be loading into memory within a certain timeframe. But PC game makers can't really trust that, so any game designed for PC probably won't operate (much) in the "3gbs expected SSD to VRAM" space. Additionally, PC motherboards and software isn't really designed for that either, becoming bottlenecks.
That may change in the future (I believe AMD is sorting towards connecting SSDs more directly to the GPU instead of the motherboard, since for gaming the vast amount of data transfer is SSD -> GPU), but with current hardware you are basically gambling that software upgrades are going to be good enough for a long time, which is always dubious.
This may change if you have a special usecase, usually from your work. If you are constantly moving very large files around, or accessing very large files (say as a video editor), then the more speed the better.
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