Black Star - Bowie. A jazz-infused, dark masterpiece with haunting vocals. Nothing to do with his death; it's a dope and clever song.
Rosemary's Baby - Fantomas. Crazy. Mike Patton humming the theme to a controversial film with Buzz from the Melvins on guitar...
Ain't That Easy - D'Angelo. His unusually layered vocal harmonies and almost off-beat music gels in a really unique way. Love him. Genius.
Bela Lugosi's Dead - Bauhaus. This is like a slowed-down Dead Kennedy's song but with gothic, swinging, cool vibes. It really culminates into a brilliant climax. One of the best songs ever.
Nannou - Aphex Twin. Nearly every aspect of the song -- percussion, melody, ambient noises -- were done on a music box.
Xen - Arca. There are fragments of motifs and phrases recognizable as music amid a mire of sordid emotions. Very clever.
Trans Europe Express - Kraftwerk. Hugely influential tune and band. Sounds like a dystopia condensed into sound. Electronic music on electricity. Meta, yo. Weird at the time, anyway.
If you like any of those, I have lots more I like. I didn't want to name too many.
Edit: Couple more.
Open Heart Zoo - Martin Grech. Gotta hear it.
Pendelous Skin - Mastodon. It turns into a gorgeous, syrupy song with gibberish (literally) lyrics at the minute mark.
Water - Yowler.
Stranger than Kindness - Nick Cave
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