Muramasa Rebirth - Technically on Wii, but that version is awful. Vita version also has 4 pieces of fantastic DLC. My favorite Vita game, bar none.
Ys: Memories of Celceta - I adore all Ys games, and this one is really good.
Soul Sacrifice: Delta - A Monster Hunter-like, except quite different with its focus on spells rather than weapons, also has a surprisingly good story.
Freedom Wars - Quite fun, if a bit forgettable.
Oreshika - A really unique JRPG, with a neat look and a fun combat system.
Tales of Hearts R - a solid Tales entry.
Hot Shots Golf - legit the best golf game ever.
Demon Gaze - one of my favorite dungeon crawlers.
Danganronpa - Only Ultimate Despair Girls is exclusive anymore, and might come to PC, but its a fun game.
Atelier Totori/Meruru Plus - the best versions of crafting focused JRPG's, that are quite fun!
Killzone Mercenary - The most technical game you will ever see, its visually amazing looks almost like a PS3 game. Decent to play.
I think the Vita has quite a few decent games, I also like the way of playing on it. Especially RPG's I think fit very, very well. Also Shiren The Wanderer is coming out on Vita in July, and I am mad hype for that.
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