Bad Company 2 and Dead Space/Dead Space 2 have already gotten several mentions. Backing those up 100%.
I recently played through Fatal Frame 2 for the first time and I thought the sound design was great. The creepy music, the light moan of wind blowing through abandoned houses, the way a ghost's voice was completely different from another's based on the way they died; the strangled schoolgirl had a raspy, quiet voice from a crushed windpipe and the drowned lady just sort of gurgles out wet, distant "help me"s.
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