For me, the best game where you can play as Superman is LEGO Batman 2 just because it plays the iconic Superman theme when you're flying around in the open world sections of Gotham City. It's a small touch, but the first time it happened, I had the biggest smile after nearly passing out from laughter since I didn't expect it. Plus, that game was actually pretty fun to get 100% achievements in (I haven't played much of most of the other LEGO games, but I've heard they're all pretty much the same aside from the licenses).
In terms of a Superman-centric game, I kinda like the idea of the Superman Returns game that came out alongside the movie where his "health" is determined by how much of Metropolis gets destroyed. If someone could make something like that, but make it better and more fun, and/or have it be a mechanic that affects Superman's morale/will to fight (which won't kill him per se, but will affect how well he fights hand-to-hand and how effective his other powers work), I could see that being fun if it's balanced correctly and fun.
Alternatively, do something like Final Fantasy II/IV where you start off as regular Clark Kent and build up your stats in terms of physical strength, speed, etc. Then, when you finally become Superman proper, those stats will be boosted compared to the others.
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