Cowboy bebop, Gurren Lagann, Golden Boy, Azumanga Daioh, Eden of the East, and Fooly Cooly for TV series. Spirited Away, Mind Game, Howl's Moving Castle, Castle in the Sky, and 5 centimeters per second for movies. All good stuff to star on!
Both Fullmetal Alchemist series are good, so is Ghost in the Shell: GiTS. I wouldn't start on them necessarily, maybe after you've gotten into it. Especially since FMA is pretty long 50+ episodes for both series.
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